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[JohnD] The relevant equation is
Qi = Cij Vj
This equation and the underlying physics is discussed at
http://www.av8n.com/physics/laplace.html#q_of_v
[Brian] Capacitance is the property of a two terminal device to store
external electrical charge whose magnitude is measured by the reciprocal
of the rate of change of voltage difference between
the terminals, which is proportional to the amplitude of a constant current
impressed between the terminals.
[JohnM] There was a discussion on Phys-L back in March of 1997 that began with a question from Ludwik titled "How many volts?" and led into this same territory.
<https://carnot.physics.buffalo.edu/archives/1997/03_1997/msg00476.html>
[Alphonsus] Actually, I guess your question is related to the "Physics Challenge".
[Mark] In your spherical capacitor example, you have to distinguish between the charge on the inner surface of the outer sphere, and the charge on the outer surface. The charge on the inner surface of the outer sphere will adjust itself to be equal to -Qa, since there can be no electrostatic field within the metal of the outer sphere. The capacitance between the inner surface of the outer sphere and the inner sphere, which is a purely geometric parameter, won't change.
But, since in this case the outer sphere is "floating" and has an excess charge on its outer surface, there also will be a capacitance between the outer surface of the outer sphere and infinity.